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Research Data for the publication titled "Impact of irradiation conditions on the magnetic field sensitivity of spin defects in hBN nano flakes"

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Version 2 2025-11-03, 12:45
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posted on 2025-11-03, 12:45 authored by Saksham MahajanSaksham Mahajan, Ravi KumarRavi Kumar, Aferdita XhameniAferdita Xhameni, Gautham Venu, Basanta Mistri, Felix DonaldsonFelix Donaldson, Takashi Taniguchi, Kenji Watanabe, Siddharth Dhomkar, Antonio LombardoAntonio Lombardo, John MortonJohn Morton
<p dir="ltr">Abstract for the paper : We study V<sub>B</sub><sup>−</sup> centres generated by helium focused ion beam (FIB) irradiation in thin (~70 nm) hBN nanoflakes, in order to investigate the effect of implantation conditions on the key parameters that influence the magnetic field sensitivity of V<sub>B</sub><sup>−</sup> quantum sensors. Using a combination of photoluminescence, optically detected magnetic resonance, and Raman spectroscopy, we examine the competing factors of maximizing signal intensity through larger V<sub>B</sub><sup>−</sup> concentration against the degradation in spin coherence and lattice quality observed at high ion fluences.Our results indicate that both the V<sub>B</sub><sup>−</sup> spin properties and hBN lattice parameters are largely preserved up to an ion fluence of 10¹⁴ ions cm⁻², beyond which significant degradation occurs in both. At the optimal implantation dose, an AC magnetic sensitivity of approximately 1 μT / √Hz is achieved. Using the patterned implantation enabled by the FIB, we find that V<sub>B</sub><sup>−</sup> centres and the associated lattice damage are well localized to the implanted regions. This work demonstrates how careful selection of fabrication parameters can be used to optimize the properties of V<sub>B</sub><sup>−</sup> centres in hBN, supporting their application as quantum sensors based in two-dimensional materials.</p>

Funding

EPSRC Hub in Quantum Computing and Simulation

Engineering and Physical Sciences Research Council

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DTP 2020-2021 University College London

Engineering and Physical Sciences Research Council

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SRG/2023/000322

Materials Synthesis for 2.5 Dimensional Structures

Japan Society for the Promotion of Science

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Exploration for quntum functions of hexagonal Boron Nitride by their defect control

Japan Society for the Promotion of Science

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Construction and application of quantum optical platform using two-dimensional semiconductor heterostructures

Japan Science and Technology Agency

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